To remove pictures from your ipod directly
- Navigate to the main Menu.
- Select Extras, then Photo Import.
- Select the roll name, then Delete Roll, and then Delete.
In iTunes
Imported photos can also be deleted from the iPod disk while it is attached to a computer.
- Connect your iPod to your computer.
- When the iPod icon appears in the iTunes Source list (below Devices), select it.
- If the Summary pane isn't showing, click the Summary tab.
- Click "Enable disk use".
- All imported photos are located in the "DCIM" folder on the iPod disk.
Source and more about it at
http://docs.info.apple.com/article.html?artnum=301111
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